It was a match made in Hollywood heaven when Brad Pitt and Angelina Jolie teamed up to star as a married couple secretly moonlighting as assassins in 2005's 'Mr. & Mrs. Smith.' The onscreen chemistry was so palpable that it wasn't long before it seeped into reality. Now, six years and six children (three adopted, three biological) later, the power couple is looking to revisit that professional partnership that started it all.

In an interview with NPR, Pitt said that the couple is looking for another onscreen collaboration.

"We're not ones to repeat ourselves, but we'd like to, because right now, we're hopscotching with films so one can be with the kids and one's free to work," Pitt said. "And why aren't we doing them together? Why aren't we doing everything together?"